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The purpose of this study was to examine the effect of the Vee Diagram, one of self-motivated learning instruments for elementary students, on their scientific attitudes, academic achievements, and scientific process skills. Results of the study were as follows: First, science lectures utilizing the Vee Diagram had significant effects on scientific attitudes. Especially, scientific attitudes including curiosities, voluntariness, activeness, and judging reservation, were meaningfully improved. Second, science lectures utilizing the Vee Diagram had significant effects on science academic achievements. Third, science lectures utilizing the Vee Diagram had significant effects on scientific process skills. In the area of basic process skills, observation and classification showed a significant results, while In the area of comprehensive process skills, data interpretation showed a significant results.